The biggest problem with carbon capture and sequestration (CCS) is that the efficiencies go down dramatically the more diluted the carbon is. So capturing CO2 at a smokestack is way more efficient than sucking it straight from the air.
-- By extrapolation, by far the most efficient form of carbon capture and sequestration would be to capture the carbon in its purest form. That is, take coal and other fossil fuels, and bury them underground!
Patrik
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